A reconfigurable and compact circular multi-pass sensor for ultra-sensitive methane detection


Kaya G., Keskin A., Kaya N.

JOURNAL OF INSTRUMENTATION, cilt.21, sa.09, ss.1-13, 2026 (SCI-Expanded, Scopus)

  • Yayın Türü: Makale / Tam Makale
  • Cilt numarası: 21 Sayı: 09
  • Basım Tarihi: 2026
  • Doi Numarası: 10.1088/1748-0221/21/09/p09049
  • Dergi Adı: JOURNAL OF INSTRUMENTATION
  • Derginin Tarandığı İndeksler: Scopus, Science Citation Index Expanded (SCI-EXPANDED), Compendex, Index Islamicus, INSPEC
  • Sayfa Sayıları: ss.1-13
  • Çanakkale Onsekiz Mart Üniversitesi Adresli: Evet

Özet

Abstract Atmospheric methane (CH 4 ) monitoring requires an optimal balance between ultra-high sensitivity and mechanical field-readiness. Conventional multi-pass architectures, such as Herriott cells, are fundamentally constrained by rigid geometries and alignment sensitivities that limit real-time optimization capability. To overcome this limitation, we introduce an angularly tunable circular multi-pass absorption cell (CMPC) integrated with digital wavelength modulation spectroscopy (WMS). By leveraging a 20 cm radius “optical cage” architecture, continuous optical path-length tunability is achieved through precise beam injection angle control, resulting in a large effective optical path length of 134.8 m via 337 reflections. Targeting the R 4 transition near 1.651 μm ensures strong spectral isolation from ambient H 2 O and CO 2 interference. The system incorporates a balanced dual-beam detection scheme that suppresses common-mode noise and laser intensity fluctuations, yielding a signal-to-noise ratio (SNR) of 180 and a short-term precision of 50.1 ppb. Allan deviation analysis confirms a detection limit of 55 ppb at 1 s integration time, reaching an ultimate precision of 6.25 ppb at an optimum integration time of 841 s. These results demonstrate that the proposed architecture provides a compact, mechanically robust, and highly sensitive alternative to conventional fixed-geometry methane sensing systems.